Unprecedented Li<sup>+</sup> Exchange in an Anionic\nMetal–Organic Framework: Significantly Enhanced Gas Uptake\nCapacity
Bo Liu (127343)Rui Zhang (13940)Chun-Yang Pan (1687216)Hai-Long Jiang (691928)
Abstract
We herein report\nthe first example of Li<sup>+</sup> exchanged with both the guest\nH<sub>2</sub>N(Me)<sub>2</sub><sup>+</sup> cations located in the\nchannels and the coordinated metal ions from an anionic metal–organic\nframework (MOF), leading to significant enhancement of the pore volume\nand gas sorption abilities of the exchanged MOF. Furthermore, both\nMOFs before and after Li<sup>+</sup> exchange show good selective\nadsorption for CO<sub>2</sub> over CH<sub>4</sub>.
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