Surface Activation of Electrocatalysis at Oxide Electrodes. Concerted Electron−Proton Transfer

Christopher J. Gagliardi (2023828); Jonah W. Jurss (2164228); H. Holden Thorp (1627792); Thomas J. Meyer (1234965)

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Surface Activation of Electrocatalysis at Oxide Electrodes. Concerted Electron−Proton Transfer

Christopher J. Gagliardi (2023828)Jonah W. Jurss (2164228)H. Holden Thorp (1627792)Thomas J. Meyer (1234965)

Year: 2016 Journal: OPAL (Open@LaTrobe) (La Trobe University) Publisher: La Trobe University

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Abstract

Dramatic rate enhancements are observed for the oxidation of phenols, including tyrosine, at indium−tin oxide electrodes modified by the addition of the electron-transfer relays [MII(bpy)2(4,4′-(HO)2P(O)CH2)2bpy)]2+ (M = Ru, Os) with clear evidence for the importance of proton-coupled electron transfer and concerted electron−proton transfer.

Keywords:

Electrocatalyst Oxide Electron transfer Catalysis Electrode

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Metal-Catalyzed Oxygenation Mechanisms

Physical Sciences → Chemistry → Inorganic Chemistry

Radical Photochemical Reactions

Physical Sciences → Chemistry → Organic Chemistry

CO2 Reduction Techniques and Catalysts

Physical Sciences → Energy → Renewable Energy, Sustainability and the Environment

Surface Activation of Electrocatalysis at Oxide Electrodes. Concerted Electron−Proton Transfer

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