Efficient Catalysis of Ammonia Borane Dehydrogenation

Melanie C. Denney (2340610); Vincent Pons (2425450); Travis J. Hebden (2319073); D. Michael Heinekey (1635046); Karen I. Goldberg (1651462)

JOURNAL ARTICLE

Efficient Catalysis of Ammonia Borane Dehydrogenation

Melanie C. Denney (2340610)Vincent Pons (2425450)Travis J. Hebden (2319073)D. Michael Heinekey (1635046)Karen I. Goldberg (1651462)

Year: 2016 Journal: OPAL (Open@LaTrobe) (La Trobe University) Publisher: La Trobe University

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Abstract

In the presence of an iridium pincer complex, dehydrogenation of ammonia borane (H3NBH3) occurs rapidly at room temperature in tetrahydrofuran to generate 1.0 equivalent of H2 and [NH2BH2]5. A metal borohydride complex has been isolated as a dormant form of the catalyst which can be reactivated by reaction with H2.

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Hydrogen Storage and Materials

Physical Sciences → Materials Science → Materials Chemistry

Boron Compounds in Chemistry

Health Sciences → Medicine → Radiology, Nuclear Medicine and Imaging

Organoboron and organosilicon chemistry

Physical Sciences → Chemistry → Organic Chemistry

Efficient Catalysis of Ammonia Borane Dehydrogenation

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