Enantioselective Hydrogenation with Chiral Frustrated Lewis Pairs

Dianjun Chen; Yutian Wang; Jürgen Klankermayer

doi:10.1002/anie.201004525

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Enantioselective Hydrogenation with Chiral Frustrated Lewis Pairs

Dianjun Chen Yutian Wang Jürgen Klankermayer

Year: 2010 Journal: Angewandte Chemie International Edition Vol: 49 (49)Pages: 9475-9478 Publisher: Wiley

DOI: 10.1002/anie.201004525

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Abstract

No subsequent frustration: Frustrated Lewis pairs (FLPs) have been recently introduced as an unprecedented possibility to activate hydrogen. On the basis of this concept the first example of highly enantioselective catalytic hydrogenation of imines using chiral FLPs has been demonstrated (see scheme).

Keywords:

Enantioselective synthesis Frustrated Lewis pair Frustration Lewis acids and bases Chemistry Materials science Catalysis Organic chemistry Physics Condensed matter physics

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Organoboron and organosilicon chemistry

Physical Sciences → Chemistry → Organic Chemistry

Boron Compounds in Chemistry

Health Sciences → Medicine → Radiology, Nuclear Medicine and Imaging

Crystallography and molecular interactions

Physical Sciences → Chemistry → Physical and Theoretical Chemistry

Enantioselective Hydrogenation with Chiral Frustrated Lewis Pairs

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