A Compactly Fused π-Conjugated Tetrathiafulvalene−Perylenediimide Donor−Acceptor Dyad
Michael Jaggi (2205154)Carmen Blum (2205160)Nathalie Dupont (1936063)Jakob Grilj (1995385)Shi-Xia Liu (827738)Jürg Hauser (1536169)Andreas Hauser (1271226)Silvio Decurtins (827737)
Abstract
The synthesis and structural characterization of a tetrathiafulvalene-fused perylenediimide molecular dyad is presented. Its largely extended π-conjugation provides intense optical absorption bands over a wide spectral range. The planar functional molecule exhibits a short-lived nonluminescent excited state attributed to intramolecular charge separation.
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