JOURNAL ARTICLE

Self-Biased High-Responsivity\nPhotodetector Based\non a Bi<sub>2</sub>SeTe<sub>2</sub> Topological Insulator

Abstract

Topological insulators\nshow promise for high-performance optoelectronic\napplications due to their nonlinear optical properties, broad spectral\nabsorption, ultrafast response to optical excitation, and excellent\nthermoelectric properties. Here, we introduce a self-biased photodetector\nbased on the topological insulator Bi<sub>2</sub>SeTe<sub>2</sub>,\ndriven by the photothermoelectric effect. Operating without external\nbias, the photodetector delivers a competitive visible-range photoresponse\nreaching responsivity of ≈27 mA/W and detectivity of ≈2\n× 10<sup>9</sup> Jones at 458 nm. Comparable to individual topological\ninsulators as well as topological insulator-based heterojunctions,\nthis underscores Bi<sub>2</sub>SeTe<sub>2</sub>’s potential,\nespecially in scenarios where external power sources cannot be used.\nIts self-biased nature eliminates the need for an external bias,\nmaking it an ideal material for low-power and remote-sensing applications.

Keywords:
Topological insulator Photodetector Ultrashort pulse Topology (electrical circuits) Nonlinear system Responsivity Nonlinear optics Insulator (electricity) Ideal (ethics)

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Topics

Topological Materials and Phenomena
Physical Sciences →  Physics and Astronomy →  Atomic and Molecular Physics, and Optics
Phase-change materials and chalcogenides
Physical Sciences →  Materials Science →  Materials Chemistry
2D Materials and Applications
Physical Sciences →  Materials Science →  Materials Chemistry

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Journal:   OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) Year: 2022
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