Boosted nitrate electroreduction to ammonia on Fe-doped SnS<sub>2</sub> nanosheet arrays rich in S-vacancies

Kai Chen; Yaojing Luo; Peng Shen; Xiaoxu Liu; Xingchuan Li; Xiaotian Li; Ke Chu

doi:10.1039/d2dt01542k

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Boosted nitrate electroreduction to ammonia on Fe-doped SnS₂ nanosheet arrays rich in S-vacancies

Kai Chen Yaojing Luo Peng Shen Xiaoxu Liu Xingchuan Li Xiaotian Li Ke Chu

Year: 2022 Journal: Dalton Transactions Vol: 51 (27)Pages: 10343-10350 Publisher: Royal Society of Chemistry

DOI: 10.1039/d2dt01542k

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Abstract

Fe–SnS 2 exhibits a high NO 3 RR activity, attributed to that S-vacancies act as the main active sites, while Fe-doping can further regulated the electronic structure of S-vacancies to optimize the binding energies of the NO 3 RR intermediates.

Keywords:

Nanosheet Density functional theory Doping Electrochemistry Materials science Ammonia Catalysis Yield (engineering) Chemical engineering Nitrate Nanotechnology Faraday efficiency Binding energy Inorganic chemistry Chemistry Physical chemistry Computational chemistry Optoelectronics Atomic physics Metallurgy Organic chemistry Electrode

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Ammonia Synthesis and Nitrogen Reduction

Physical Sciences → Chemical Engineering → Catalysis

Advanced Photocatalysis Techniques

Physical Sciences → Energy → Renewable Energy, Sustainability and the Environment

Caching and Content Delivery

Physical Sciences → Computer Science → Computer Networks and Communications

Boosted nitrate electroreduction to ammonia on Fe-doped SnS₂ nanosheet arrays rich in S-vacancies

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