Ultrafast stimulated emission microscopy of single nanocrystals

Abstract

Tracking excitations Illumination can be used to excite a sample from its ground state to a number of excited states. Typically, however, the details of the excitation dynamics are hidden from view because they decay so fast. Piatkowski et al. combined pump-probe transient absorption and two-pulse photoluminescence correlation spectroscopy, allowing them to assess stimulated emission and ground-state bleaching contributions to the transient absorption signal. This approach provides a window on the excitation dynamics within single nanocrystals and should also be useful for ultrafast nanocharacterization of complex samples. Science , this issue p. 1240