Spectral broadening effects on metal photoemission by femtosecond laser pulses

Abstract

Emitted electronic densities from an Al surface have been computed for various temporal shapes of near-infrared femtosecond laser pulses (less than or equal to 20 fs) over a wide range of low and intermediate laser intensities. At low intensities photoemission originates from the high-energy tail of the pulse spectrum leading to linear absorption in all cases, even if several photons are necessary to eject an electron at higher intensities. We propose an analytical method to calculate the transition intensity in which the behavior of emitted densities evolves from the single-photon ${I}_{m}$ slope to the multiphoton ${I}_{m}^{n}$ one (with ${I}_{m}$ the maximum intensity and $n$ the number of absorbed photons). We show that the use of a flat-top profile or at least of a super-Gaussian envelope enables strong electron emission at very low intensities for realistic pulse durations and should allow experimental observation of the transition between these two regimes of photoemission.