Hydrogenation of carbon dioxide to methanol using a homogeneous ruthenium–Triphos catalyst: from mechanistic investigations to multiphase catalysis

Sebastian Wesselbaum; Verena Moha; Markus Meuresch; Sandra Brosinski; Katharina Thenert; Jens Kothe; Thorsten vom Stein; Ulli Englert; Markus Hölscher; Jürgen Klankermayer; Walter Leitner

doi:10.1039/c4sc02087a

JOURNAL ARTICLE

Hydrogenation of carbon dioxide to methanol using a homogeneous ruthenium–Triphos catalyst: from mechanistic investigations to multiphase catalysis

Sebastian Wesselbaum Verena Moha Markus Meuresch Sandra Brosinski Katharina Thenert Jens Kothe Thorsten vom Stein Ulli Englert Markus Hölscher Jürgen Klankermayer Walter Leitner

Year: 2014 Journal: Chemical Science Vol: 6 (1)Pages: 693-704 Publisher: Royal Society of Chemistry

DOI: 10.1039/c4sc02087a

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Abstract

The hydrogenation of CO₂ to methanol using a recyclable molecular organometallic catalyst in the absence of an alcohol additive is demonstrated for the first time.

Keywords:

Triphos Ruthenium Catalysis Methanol Homogeneous Carbon dioxide Homogeneous catalysis Chemistry Materials science Chemical engineering Organic chemistry Thermodynamics Physics Engineering

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Carbon dioxide utilization in catalysis

Physical Sciences → Chemical Engineering → Process Chemistry and Technology

Catalysts for Methane Reforming

Physical Sciences → Chemical Engineering → Catalysis

Catalysis for Biomass Conversion

Physical Sciences → Engineering → Biomedical Engineering

Hydrogenation of carbon dioxide to methanol using a homogeneous ruthenium–Triphos catalyst: from mechanistic investigations to multiphase catalysis

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